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Reference: Koelman P.M.J., Heijkers S., Mousavi S.T., Greaf W., Mihailova D., Kozak T., Bogaerts A. and van Dijk J. (2016). A Comprehensive Chemical Model for the Splitting of CO2 in Non-Equilibrium Plasmas. Plasma Processes and Polymers, DOI:10.1002/ppap.201600155. [ bib | http ]
Abstract: In this work an extensive chemical model is presented for a CO2 plasma that is relevant for the production of `solar fuels'. It consists of 72 species and 5732 reactions. It is based on species definitions and reaction rate coefficients from previous literature, which have been rigorously reviewed, and is augmented with reaction rate coefficients that are obtained from the application of scaling laws. The input data set, which is suitable for usage with the plasma simulation software PLASIMO has been made available in human-readable electronic form on the publisher's website. The correctness of this implementation of the model has been established by realizing an independent ZDPlasKin - compatible implementation setting up equivalent physical models and verifying that the results agree. Results of these `global models' are presented for a typical case study, a cylindrical DBD plasma reactor with pulsed power input.
The archives koelman2016.tgz and koelman.zip contain the data that are
used in this paper.
The ZIP file has the CRLF line endings and is suitable for Windows systems,
the tgz archive is meant for Unix/Linux systems. Both archives contain only
human-readable text files and unpack to a subdirectory koelman2016.
If you wish to use these data with your copy of the PLASIMO plasma modelling toolkit, please unpack the archive relative to the input directory of your PLASIMO installation.